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Phys. Rev. E 80, 026401 (2009) [6 pages]

Time-resolved fluorescence spectroscopy of two-photon laser-excited 8p, 9p, 5f, and 6f levels in neutral xenon

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Christoph Eichhorn1,*, Stephan Fritzsche2,3, Stefan Löhle1, Andreas Knapp1, and Monika Auweter-Kurtz4
1Institut für Raumfahrtsysteme, Universität Stuttgart, Pfaffenwaldring 31, D-70569 Stuttgart, Germany
2Gesellschaft für Schwerionenforschung (GSI), D-64291 Darmstadt, Germany
3Department of Physical Sciences, University of Oulu, P.O. Box 3000, Oulu Fin-90014, Finland
4Universität Hamburg, Edmund-Siemers Allee 1, D-20196 Hamburg, Germany

Received 14 April 2009; published 6 August 2009

Laser-induced fluorescence of two-photon excited 8p, 9p, J=0,2 and 5f, 6f, J=2 levels in neutral xenon has been investigated in the pressure regime between 4 and 120 Pa. Radiative lifetimes and collisional deactivation rates have been deduced especially for the 5f[3/2]2, 5f[5/2]2, and 8p[1/2]0 levels using the Stern-Volmer approach. The spontaneous lifetimes for 5f[3/2]2, 5f[5/2]2, and 8p[1/2]0 levels are 94, 78, and 207 ns, respectively. These lifetimes have been calculated also by applying extended multiconfiguration Dirac-Fock wave functions and are found in agreement with experiment within 10–25 %.

© 2009 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevE.80.026401
DOI:
10.1103/PhysRevE.80.026401
PACS:
52.38.−r, 32.80.Rm, 32.70.Cs

*eichhorn@irs.uni-stuttgart.de