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Phys. Rev. E 68, 041110 (2003) [7 pages]

Relationship between dynamical heterogeneities and stretched exponential relaxation

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S. I. Simdyankin1,2 and Normand Mousseau2
1Department of Chemistry, University of Cambridge, Lensfield Road, Cambridge CB2 1EW, United Kingdom
2Département de Physique and Centre de Recherche en Physique et Technologie des Couches Minces, Université de Montréal, Case Postale 6128, succursale Centre-ville, Montréal, Québec, Canada, H3C 3J7

Received 16 May 2003; revised 11 August 2003; published 27 October 2003

We identify dynamical heterogeneities as an essential prerequisite for stretched exponential relaxation in dynamically frustrated systems. This heterogeneity takes the form of ordered domains of finite but diverging lifetime for particles in atomic or molecular systems, or spin states in magnetic materials. At the onset of the dynamical heterogeneity, the distribution of time intervals spent in such domains or traps becomes stretched exponential at long times. We rigorously show that once this is the case the autocorrelation function of the renewal process formed by these time intervals is also a stretched exponential at long times.

© 2003 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevE.68.041110
DOI:
10.1103/PhysRevE.68.041110
PACS:
05.20.-y, 61.20.Lc, 05.45.-a, 61.43.Fs