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Phys. Rev. E 63, 031206 (2001) [9 pages]

Criterion for determining clustering versus reentrant melting behavior for bounded interaction potentials

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C. N. Likos1,*, A. Lang1,2, M. Watzlawek1,†, and H. Löwen1
1Institut für Theoretische Physik II, Heinrich-Heine-Universität Düsseldorf, Universitätsstraße 1, D-40225 Düsseldorf, Germany
2Institut für Theoretische Physik and CMS, Technische Universität Wien, Wiedner Hauptstraße 8-10, A-1040 Wien, Austria

Received 29 March 2000; revised 16 October 2000; published 27 February 2001

We examine in full generality the phase behavior of systems whose constituent particles interact by means of potentials that do not diverge at the origin, are free of attractive parts, and decay fast enough to zero as the interparticle separation r goes to infinity. By employing a mean field-density functional theory which is shown to become exact at high temperatures and/or densities, we establish a criterion that determines whether a given system will freeze at all temperatures or it will display reentrant melting and an upper freezing temperature.

© 2001 The American Physical Society

URL:
http://link.aps.org/doi/10.1103/PhysRevE.63.031206
DOI:
10.1103/PhysRevE.63.031206
PACS:
61.20.Gy, 64.70.-p

*Email address: likos@thphy.uni-duesseldorf.de

Present address: Bayer AG, Central Research Division, D-51368 Leverkusen, Germany